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196
result(s) for
"mode hybridization"
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Active coherent control of nanoscale light confinement:Modulation of plasmonic modes and position of hotspots for surface-enhanced Raman scattering detection
by
Zhendong Zhu;Qixia Wang;Fa Zeng;Oubo You;Sitian Gao;Benfeng Bai;Qiaofeng Tan;Guofan Jin;Qunqing Li;Shoushan Fan;Wei Li;Yushu Shi;Xueshen Wang
in
Active control
,
Atomic/Molecular Structure and Spectra
,
Biomedicine
2017
Multistep plasmonic nanostructures can induce the deep modulation ofelectromagnetic-field interactions on the nanoscale for positioning hotspots,and this generation of enhanced fields is important in many optical applications.In this article, a new strategy is proposed for fabricating a plasmonic double-stacked nanocone (DSC) nanostructure. In the DSC structure, a tunable plasmonichybrid mode proceeds from the strong coupling of the plasmonic resonance ofa fundamental cavity mode with a localized surface plasmon gap mode. In thenanostructure, the far-field response is deeply modulated and the hottest spotscan be effectively positioned on the top surface of the DSC nanostructure. Acontrollable and cost-effective mask-reconfiguration technique for manufacturingthe multiscale nanostructure is developed, which guarantees the generation ofthe introduced crucial stage on the DSC nanostructure. To evaluate the features ofthe plasmonic resonance, the DSC nanostructure is used as a surface-enhancedRaman scattering (SERS) substrate for detecting 4-mercaptopyridine moleculesunder specific excitation conditions. Its good performance, with an averagemeasured SERS enhancement factor as high as 108,
Journal Article
Polarization-Insensitive Waveguide Schottky Photodetectors Based on Mode Hybridization Effects in Asymmetric Plasmonic Waveguides
2020
Two types of configurations are theoretically proposed to achieve high responsivity polarization-insensitive waveguide Schottky photodetectors, i.e., a dual-layer structure for 1.55 µm and a single-layer structure for 2 µm wavelength band. Mode hybridization effects between quasi-TM modes and sab1 modes in plasmonic waveguides are first presented and further investigated under diverse metal types with different thicknesses in this work. By utilizing the mode hybridization effects between quasi-TE mode and aab0 mode, and also quasi-TM and sab1 mode in our proposed hybrid plasmonic waveguide, light absorption enhancement can be achieved under both TE and TM incidence within ultrathin and short metal stripes, thus resulting in a considerable responsivity for Si-based sub-bandgap photodetection. For 1.55 µm wavelength, the Au-6 nm-thick device can achieve absorptance of 99.6%/87.6% and responsivity of 138 mA·W−1/121.2 mA·W−1 under TE/TM incidence. Meanwhile, the Au-5 nm-thick device can achieve absorptance of 98.4%/90.2% and responsivity of 89 mA·W−1/81.7 mA·W−1 under TE/TM incidence in 2 µm wavelength band. The ultra-compact polarization-insensitive waveguide Schottky photodetectors may have promising applications in large scale all-Si photonic integrated circuits for high-speed optical communication.
Journal Article
Acoustic Skyrmionic Mode Coupling and Transferring in a Chain of Subwavelength Metastructures
2024
Skyrmions, a stable topological vectorial textures characteristic with skyrmionic number, hold promise for advanced applications in information storage and transmission. While the dynamic motion control of skyrmions has been realized with various techniques in magnetics and optics, the manipulation of acoustic skyrmion has not been done. Here, the propagation and control of acoustic skyrmion along a chain of metastructures are shown. In coupled acoustic resonators made with Archimedes spiral channel, the skyrmion hybridization is found giving rise to bonding and antibonding skyrmionic modes. Furthermore, it is experimentally observed that the skyrmionic mode of acoustic velocity field distribution can be robustly transferred covering a long distance and almost no distortion of the skyrmion textures in a chain of metastructures, even if a structure defect is introduced in the travel path. The proposed localized acoustic skyrmionic mode coupling and propagating is expected in future applications for manipulating acoustic information storage and transfer. The propagation and control of acoustic skyrmion along a chain of metastructures is proposed. The metastructure made with Archimedes spiral channel, the skyrmion hybridization is presented between neighboring structures. Then, it is experimentally observed that the skyrmionic mode of acoustic velocity field distribution can be robustly transferred covering a long distance, even if some structure defects are introduced in the travel path.
Journal Article
Multiresonant plasmonics with spatial mode overlap: overview and outlook
2019
Plasmonic nanostructures can concentrate light and enhance light-matter interactions in the subwavelength domain, which is useful for photodetection, light emission, optical biosensing, and spectroscopy. However, conventional plasmonic devices and systems are typically optimized for the operation in a single wavelength band and thus are not suitable for multiband nanophotonics applications that either prefer nanoplasmonic enhancement of multiphoton processes in a quantum system at multiple resonant wavelengths or require wavelength-multiplexed operations at nanoscale. To overcome the limitations of “single-resonant plasmonics,” we need to develop the strategies to achieve “multiresonant plasmonics” for nanoplasmonic enhancement of light-matter interactions at the same locations in multiple wavelength bands. In this review, we summarize the recent advances in the study of the multiresonant plasmonic systems with spatial mode overlap. In particular, we explain and emphasize the method of “plasmonic mode hybridization” as a general strategy to design and build multiresonant plasmonic systems with spatial mode overlap. By closely assembling multiple plasmonic building blocks into a composite plasmonic system, multiple nonorthogonal elementary plasmonic modes with spectral and spatial mode overlap can strongly couple with each other to form multiple spatially overlapping new hybridized modes at different resonant energies. Multiresonant plasmonic systems can be generally categorized into three types according to the localization characteristics of elementary modes before mode hybridization, and can be based on the optical coupling between: (1) two or more localized modes, (2) localized and delocalized modes, and (3) two or more delocalized modes. Finally, this review provides a discussion about how multiresonant plasmonics with spatial mode overlap can play a unique and significant role in some current and potential applications, such as (1) multiphoton nonlinear optical and upconversion luminescence nanodevices by enabling a simultaneous enhancement of optical excitation and radiation processes at multiple different wavelengths and (2) multiband multimodal optical nanodevices by achieving wavelength multiplexed optical multimodalities at a nanoscale footprint.
Journal Article
Polarization Analysis of Vertically Etched Lithium Niobate-on-Insulator (LNOI) Devices
2024
LNOI devices have emerged as prominent contributors to photonic integrated circuits (PICs), benefiting from their outstanding performance in electro-optics, acousto-optics, nonlinear optics, etc. Due to the physical properties and current etching technologies of LiNbO3, slanted sidewalls are typically formed in LNOI waveguides, causing polarization-related mode hybridization and crosstalk. Despite the low losses achieved with fabrication advancements in LNOI, such mode hybridization and crosstalk still significantly limit the device performance by introducing polarization-related losses. In this paper, we propose a vertically etched LNOI construction. By improving the geometrical symmetry in the waveguides, vertical sidewalls could adequately mitigate mode hybridization in common waveguide cross sections. Taking tapers and bends as representatives of PIC components, we then conducted theoretical modeling and simulations, which showed that vertical etching effectively exempts devices from polarization-related mode crosstalk. This not only improves the polarization purity and input mode transmittance but also enables lower polarization-related losses within more compact structures. As a demonstration of fabrication feasibility, we innovatively proposed a two-step fabrication technique, and successfully fabricated waveguides with vertical sidewalls. Such vertical etching technology facilitates the development of next-generation high-speed modulators, nonlinear optical devices, and other advanced photonic devices with lower losses and a smaller footprint, driving further innovations in both academic research and industrial applications.
Journal Article
The Hybridization of Fabry–Perot and Tamm Modes in a Spatially Inhomogeneous Magneto-Photonic Crystal
2024
Results are presented from studying features of the excitation of different resonant modes in a spatially non-homogeneous magnetophotonic crystal with a plasmonic coating. It is shown that several resonant Fabry–Perot modes and the Tamm plasmon mode are generated in such a crystal. Due to the inhomogeneity of the structure, these modes undergo a spectral shift within the photonic band gap upon changing the thickness of the layers that make up the magnetophotonic crystal.
Journal Article
Effect of Process Parameters on Mode Conversion in Submicron Tapered Silicon Ridge Waveguides
2021
The modal property and light propagation in tapered silicon ridge waveguides with different ridge heights are investigated for a silicon on insulator (SOI) platform with a 500 nm silicon (Si) thickness. Mode conversion between the transverse magnetic (TM) fundamental and higher-order transverse electric (TE) modes occurs when light is propagated in a waveguide taper. Such a conversion is due to mode hybridization resulting from the vertical asymmetry of the cross-section in the ridge waveguides. The influence of angled sidewalls and asymmetric cladding on mode conversion is also studied. It is shown that a very long taper length (adiabatic) is required for a complete conversion to take place. Conversely, such mode conversion could be suppressed by designing a short non-adiabatic taper. Our results show that significant improvement in performance metrics can be achieved by considering process parameters’ effect on mode conversion. With an optimum selection of the etching depth and accounting asymmetries due to angled sidewalls and cladding, we demonstrate an 84.7% reduction in taper length (adiabatic) for mode conversion and a 97% efficiency TM preserving taper (ultra-short). The analysis is essential for applications such as compact polarizers, polarization splitters/rotators, and tapers for TM devices.
Journal Article
Hybridization of Surface Plasmon Polariton and Photonic Crystal Modes in Bragg Mirror with Periodically Profiled Metal Film
by
Sosnova, Mariya V.
,
Dmitruk, Nicolas L.
,
Mamykin, Sergii V.
in
Bragg reflectors
,
Chemistry and Materials Science
,
Corrugating
2016
The hybridization of the plasmonic and guided modes in the case of one-dimension photonic crystal based on Bragg mirror terminated by a corrugated metal film has been demonstrated theoretically. The simulations have showed that the hybrid plasmonic-photonic mode is characterized by low broadening due to redistribution of the electric field intensity between photonic mode and surface plasmon polariton. It was found that the
Q
-factor and the polarisation sensitivity of these modes are about 144 and 25, respectively, that is 3 times greater than for surface plasmon polariton exciting in similar structure without Bragg mirror.
Journal Article
Shining light on the microscopic resonant mechanism responsible for cavity-mediated chemical reactivity
by
Flick, Johannes
,
Ronca, Enrico
,
Rubio, Angel
in
639/638/440/950
,
639/766/400/2797
,
639/766/483/1139
2022
Strong light–matter interaction in cavity environments is emerging as a promising approach to control chemical reactions in a non-intrusive and efficient manner. The underlying mechanism that distinguishes between steering, accelerating, or decelerating a chemical reaction has, however, remained unclear, hampering progress in this frontier area of research. We leverage quantum-electrodynamical density-functional theory to unveil the microscopic mechanism behind the experimentally observed reduced reaction rate under cavity induced resonant vibrational strong light-matter coupling. We observe multiple resonances and obtain the thus far theoretically elusive but experimentally critical resonant feature for a single strongly coupled molecule undergoing the reaction. While we describe only a single mode and do not explicitly account for collective coupling or intermolecular interactions, the qualitative agreement with experimental measurements suggests that our conclusions can be largely abstracted towards the experimental realization. Specifically, we find that the cavity mode acts as mediator between different vibrational modes. In effect, vibrational energy localized in single bonds that are critical for the reaction is redistributed differently which ultimately inhibits the reaction.
Hybridization of dark optical cavity modes with vibrational states of molecules can alter chemical reactions. Here, the authors use ab-initio methods to shine light on the associated mechanism and highlight the role of the optical mode to redistribute the vibrational energy.
Journal Article
Zr‐MOF Carrier‐Enhanced Dual‐Mode Biosensing Platforms for Rapid and Sensitive Diagnosis of Mpox
by
Zheng, Judun
,
Lin, Jingyan
,
Zhang, Mingxia
in
Acids
,
amplification‐free
,
Biosensing Techniques - methods
2024
Dual‐mode readout platforms with colorimetric and electrochemiluminescence (ECL) signal enhancement are proposed for the ultrasensitive and flexible detection of the monkeypox virus (MPXV) in different scenes. A new nanotag, Ru@U6‐Ru/Pt NPs is constructed for dual‐mode platforms by integrating double‐layered ECL luminophores and the nanozyme using Zr‐MOF (UiO‐66‐NH2) as the carrier, which not only generates enhanced ECL and colorimetric signals but also provide greater stability than that of commonly used nanotags. Dual‐mode platforms are used within 15 min from the “sample in” to the “result out” steps, without nucleic acid amplification. The colorimetric mode allows the screening of MPXV with the visual limit of detection (vLOD) of 0.1 pM (6 × 108 copies µL−1) and the ECL mode supports quantitative detection of MPXV with an LOD as low as 10 aM (6 copies·µL−1), resulting in a broad sensing range of 60 to 3 × 1011 copies·µL−1 (10 orders of magnitude). Validation is conducted using 50 clinical samples, which is 100% concordant to those of quantitative polymerase chain reaction (qPCR), indicating that Ru@U6‐Ru/Pt NPs‐based dual‐mode sensing platforms showed great promise as rapid, sensitive, and accurate tools for diagnosis of the nucleic acid of MPXV and other infectious pathogens. A new nanotag, Ru@U6‐Ru/Pt NPs is constructed for dual‐mode platforms by integrating double‐layered electrochemiluminescence luminophores and the nanozyme using Zr‐MOF as the carrier. This dual‐mode sensing platform shows great promise as a rapid, sensitive, and accurate tool for point‐of‐care testing and clinical diagnosis of nucleic acids of monkeypox virus and other infectious pathogens.
Journal Article