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"nanophotonics"
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Light-emitting metasurfaces
Photonic metasurfaces, that is, two-dimensional arrangements of designed plasmonic or dielectric resonant scatterers, have been established as a successful concept for controlling light fields at the nanoscale. While the majority of research so far has concentrated on passive metasurfaces, the direct integration of nanoscale emitters into the metasurface architecture offers unique opportunities ranging from fundamental investigations of complex light-matter interactions to the creation of flat sources of tailored light fields. While the integration of emitters in metasurfaces as well as many fundamental effects occurring in such structures were initially studied in the realm of nanoplasmonics, the field has recently gained significant momentum following the development of Mie-resonant dielectric metasurfaces. Because of their low absorption losses, additional possibilities for emitter integration, and compatibility with semiconductor-based light-emitting devices, all-dielectric systems are promising for highly efficient metasurface light sources. Furthermore, a flurry of new emission phenomena are expected based on their multipolar resonant response. This review reports on the state of the art of light-emitting metasurfaces, covering both plasmonic and all-dielectric systems.
Journal Article
Broadband high-efficiency dielectric metasurfaces for the visible spectrum
Metasurfaces are planar optical elements that hold promise for overcoming the limitations of refractive and conventional diffractive optics. Original dielectric metasurfaces are limited to transparency windows at infrared wavelengths because of significant optical absorption and loss at visible wavelengths. Thus, it is critical that new materials and nanofabrication techniques be developed to extend dielectric metasurfaces across the visible spectrum and to enable applications such as high numerical aperture lenses, color holograms, and wearable optics. Here, we demonstrate high performance dielectric metasurfaces in the form of holograms for red, green, and blue wavelengths with record absolute efficiency (>78%). We use atomic layer deposition of amorphous titanium dioxide with surface roughness less than 1 nmand negligible optical loss. We use a process for fabricating dielectric metasurfaces that allows us to produce anisotropic, subwavelength-spaced dielectric nanostructures with shape birefringence. This process is capable of realizing any high-efficiency metasurface optical element, e.g., metalenses and axicons.
Journal Article
Control of work functions of nanophotonic components
Work function is an essential material’s property playing important roles in electronics, photovoltaics, and more recently, in nanophotonics. We have studied effects of organic, and inorganic dielectric materials on work functions of Au films in single layered, and multilayered structures. We found that measured work function of metallic surfaces can be affected by dielectric materials situated 10–100 nm away from the metallic surface. We have found that, (i) the glass underneath 50 nm gold slab reduces the work function of gold, (ii) Rh590:PMMA increases the work function of a gold film deposited on top of the polymer, and (iii) reduces it if Rh590:PMMA is deposited on top of Au. (iv) With increase of the Rh590 concentration in PMMA, n, the work function first decreases (at n < 64 g/l), and then increases (at n > 64 g/l). (v) The work function of a Fabry–Perot cavity or an MIM waveguide is almost the same as that of single Au films of comparable thickness. The experimental results can be qualitatively explained in terms of a simple model taking into account adhesion of charged molecules to a metallic surface, and formation of a double layer of charges accelerating or decelerating electrons exiting the metal and decreasing or increasing the work function.
Journal Article
Atom–atom interactions around the band edge of a photonic crystal waveguide
Tailoring the interactions between quantum emitters and single photons constitutes one of the cornerstones of quantum optics. Coupling a quantum emitter to the band edge of a photonic crystal waveguide (PCW) provides a unique platform for tuning these interactions. In particular, the cross-over from propagating fields
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within the bandgap should be accompanied by a transition from largely dissipative atom–atom interactions to a regime where dispersive atom–atom interactions are dominant. Here, we experimentally observe this transition by shifting the band edge frequency of the PCW relative to the D₁ line of atomic cesium for N̄ = 3.0 ± 0.5 atoms trapped along the PCW. Our results are the initial demonstration of this paradigm for coherent atom–atom interactions with low dissipation into the guided mode.
Journal Article
Harmonic generation with multi-layer dielectric metasurfaces
Metasurfaces have recently gained extensive interest because of their extraordinary optical behavior as artificial material interfaces with ultrahigh compactness. In this framework, dielectric platforms have newly become very promising for nonlinear nanophotonics, providing opportunities, especially for ultrafast optical switching, and high harmonic generation, opening the research field of nonlinear metaoptics. Up to now, nonlinear metaoptics have been mostly explored using single metasurfaces. However, in a long-term vision, the stacking of optical metasurfaces, very challenging in terms of fabrication, is one key goal of this research field. Here, we demonstrate a three-layer metasurface in the AlGaAs-on-insulator platform, which improves the second harmonic generation efficiency by more than one order of magnitude with respect to its one-layer counterpart. Our achievement paves the way toward phase-shaping multilayer and multifunctional all-dielectric metasurfaces.
Journal Article
Nanophotonics-enabled solar membrane distillation for off-grid water purification
With more than a billion people lacking accessible drinking water, there is a critical need to convert nonpotable sources such as seawater to water suitable for human use. However, energy requirements of desalination plants account for half their operating costs, so alternative, lower energy approaches are equally critical. Membrane distillation (MD) has shown potential due to its low operating temperature and pressure requirements, but the requirement of heating the input water makes it energy intensive. Here, we demonstrate nanophotonics-enabled solar membrane distillation (NESMD), where highly localized photothermal heating induced by solar illumination alone drives the distillation process, entirely eliminating the requirement of heating the input water. Unlike MD, NESMD can be scaled to larger systems and shows increased efficiencies with decreased input flow velocities. Along with its increased efficiency at higher ambient temperatures, these properties all point to NESMD as a promising solution for household- or community-scale desalination.
Journal Article
Single photon emitters in hexagonal boron nitride: A review of progress
This report summarizes progress made in understanding properties such as zero-phonon-line energies, emission and absorption polarizations, electron-phonon couplings, strain tuning and hyperfine coupling of single photon emitters in hexagonal boron nitride. The primary aims of this research are to discover the chemical nature of the emitting centres and to facilitate deployment in device applications. Critical analyses of the experimental literature and data interpretation, as well as theoretical approaches used to predict properties, are made. In particular, computational and theoretical limitations and challenges are discussed, with a range of suggestions made to overcome these limitations, striving to achieve realistic predictions concerning the nature of emitting centers. A symbiotic relationship is required in which calculations focus on properties that can easily be measured, whilst experiments deliver results in a form facilitating mass-produced calculations.
Paper
Doping-driven topological polaritons in graphene/α-MoO3 heterostructures
Control over charge carrier density provides an efficient way to trigger phase transitions and modulate the optoelectronic properties of materials. This approach can also be used to induce topological transitions in the optical response of photonic systems. Here we report a topological transition in the isofrequency dispersion contours of hybrid polaritons supported by a two-dimensional heterostructure consisting of graphene and α-phase molybdenum trioxide. By chemically changing the doping level of graphene, we observed that the topology of polariton isofrequency surfaces transforms from open to closed shapes as a result of doping-dependent polariton hybridization. Moreover, when the substrate was changed, the dispersion contour became dominated by flat profiles at the topological transition, thus supporting tunable diffractionless polariton propagation and providing local control over the optical contour topology. We achieved subwavelength focusing of polaritons down to 4.8% of the free-space light wavelength by using a 1.5-μm-wide silica substrate as an in-plane lens. Our findings could lead to on-chip applications in nanoimaging, optical sensing and manipulation of energy transfer at the nanoscale.
Polaritonic topological transitions of the isofrequency dispersion contour are observed in a graphene/α-MoO
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heterostructure by tuning the graphene doping level, which enables partial focusing at deep subwavelength.
Journal Article