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Electronic transport properties of spin-crossover polymer plus polyaniline composites with Fe 3 O 4 nanoparticles
Electronic transport properties of spin-crossover polymer plus polyaniline composites with Fe 3 O 4 nanoparticles
by McElveen, Kayleigh A , Viswan, Gauthami , Zielinski, Ruthi , N’Diaye, Alpha T , Dowben, Peter A , Chin, WaiKiat , Mishra, Esha , Ekanayaka, Thilini K , Zaz, M Zaid , Lai, Rebecca Y , Streubel, Robert , Shapiro, David
2024
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Electronic transport properties of spin-crossover polymer plus polyaniline composites with Fe 3 O 4 nanoparticles
by McElveen, Kayleigh A , Viswan, Gauthami , Zielinski, Ruthi , N’Diaye, Alpha T , Dowben, Peter A , Chin, WaiKiat , Mishra, Esha , Ekanayaka, Thilini K , Zaz, M Zaid , Lai, Rebecca Y , Streubel, Robert , Shapiro, David
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2024
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Electronic transport properties of spin-crossover polymer plus polyaniline composites with Fe 3 O 4 nanoparticles
Electronic transport properties of spin-crossover polymer plus polyaniline composites with Fe 3 O 4 nanoparticles
by McElveen, Kayleigh A , Viswan, Gauthami , Zielinski, Ruthi , N’Diaye, Alpha T , Dowben, Peter A , Chin, WaiKiat , Mishra, Esha , Ekanayaka, Thilini K , Zaz, M Zaid , Lai, Rebecca Y , Streubel, Robert , Shapiro, David
2024

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Electronic transport properties of spin-crossover polymer plus polyaniline composites with Fe 3 O 4 nanoparticles
Electronic transport properties of spin-crossover polymer plus polyaniline composites with Fe 3 O 4 nanoparticles
Journal Article

Electronic transport properties of spin-crossover polymer plus polyaniline composites with Fe 3 O 4 nanoparticles

McElveen, Kayleigh A,
Viswan, Gauthami,
Zielinski, Ruthi,
N’Diaye, Alpha T,
Dowben, Peter A,
Chin, WaiKiat,
Mishra, Esha,
Ekanayaka, Thilini K,
Zaz, M Zaid,
Lai, Rebecca Y,
Streubel, Robert,
Shapiro, David
2024
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Overview
Adding Fe 3 O 4 nanoparticles to composites of [Fe(Htrz) 2 (trz)](BF 4 ) spin-crossover polymer and polyaniline (PANI) drives a phase separation of both and restores the molecular structure and cooperative effects of the spin-crossover polymer without compromising the increased conductivity gained through the addition of PANI. We observe an increased on-off ratio for the DC conductivity owing to an enlarged off state resistivity and a 20 times larger AC conductivity of the on state compared with DC values. The Fe 3 O 4 nanoparticles, primarily confined to the [Fe(Htrz) 2 (trz)](BF 4 ) phase, are ferromagnetically coupled to the local moment of the spin-crossover molecule suggesting the existence of an exchange interaction between both components.
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