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Degradation of tetracycline by a novel MIL-101(Fe)/TiO2 composite with persulfate
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Degradation of tetracycline by a novel MIL-101(Fe)/TiO2 composite with persulfate
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Journal Article
Degradation of tetracycline by a novel MIL-101(Fe)/TiO2 composite with persulfate
2019
Overview
An effective catalyst of MIL-101(Fe)/TiO
2
composite was synthesized by solvothermal method. The resultant MIL-101(Fe)/TiO
2
was used for advanced oxidation degradation of tetracycline (TC) for the first time. The results indicated that the MIL-101(Fe)/TiO
2
showed higher TC degradation efficiency than pure MIL-101(Fe) or TiO
2
with the persulfate. Using 1 g L
−1
MIL-101(Fe)/TiO
2
and persulfate at pH 7, 90.15% degradation rate was achieved under xenon lamp irradiation in 5 min for 20 mg L
−1
TC. TiO
2
introduced in the composite played an important role in the degradation process, in which TiO
2
had a synergetic effect with Fe
3+
to generate Fe
2+
, Ti
3+
and radicals. Fe
2+
reacted with persulfate to produce Fe
3+
and a number of
·
OH to degrade TC. This reaction process was so fast that MIL-101(Fe)/TiO
2
with persulfate could degrade TC fairly rapidly. A novel TiO
2
-based metal–organic frameworks (MOFs) composite was more efficient for degrading pharmaceutical wastewater.
Publisher
Springer US,Springer Nature B.V
