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Selective N2O Removal from the Process Gas of Nitric Acid Plants Over Ceramic 12CaO · 7Al2O3 Catalyst
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Journal Article
Selective N2O Removal from the Process Gas of Nitric Acid Plants Over Ceramic 12CaO · 7Al2O3 Catalyst
2008
Overview
Catalytic high temperature decomposition (secondary abatement) of nitrous oxide over calcium aluminate 12CaO · 7Al
2
O
3
(mayenite) was studied in the model laboratory tests (TPSR) and pilot units (steady-state) using the real feed. X-ray diffraction (XRD), scanning electron microscopy (SEM), N
2
-sorption (BET), electron paramagnetic resonance (EPR) and Raman spectroscopies were used to characterize the synthesized material. The catalyst exhibited high efficiency and selectivity in N
2
O removal, reaching practically 100% conversion at 1150 K without appreciable total losses of NO
x
. Owing to its high thermal stability and resistivity to sintering and low cost of production raw materials, mayenite was found to be a promising catalyst for economically appealing secondary abatement of nitrous oxide in nitric acid plants.
Publisher
Springer US,Springer,Springer Nature B.V
