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X-Ray FEL-induced Double Core-Hole Formation in Polyatomic Molecules

by Juranic, P , Berrah, N , Murphy, B , Prince, K. C , Piancastelli, M. N , Larsson, M , Kukk, E , Tashir, M , Osipov, T , Wada, S , Salén, P , Meulen, P. van der , Bostedt, C , Feifel, R , TARANTELLI, Francesco , Thomas, R. D , Fang, L , Ueda, K , Richter, R , Bozek, J. D , Schmidt, H. T , Ehara, M

in Auger spectrum; Core-hole state; Experimental spectra; Focal spot size; Polyatomic molecules; Pulse durations; Soft x-ray pulse; Two photon; X-ray free electron lasers; Carbon dioxide; Free electron lasers; Molecules; Photoelectron spectroscopy / Augers / Carbon dioxide / Formations / Free electron lasers / Photoelectrons / Photons / Physics / Polyatomic molecules / Pulse duration / Soft x rays / Spectra / X ray absorption / X-rays

2012

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X-Ray FEL-induced Double Core-Hole Formation in Polyatomic Molecules

2012

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2012

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Journal Article

X-Ray FEL-induced Double Core-Hole Formation in Polyatomic Molecules

Juranic, P,

Berrah, N,

Murphy, B,

Prince, K. C,

Piancastelli, M. N,

Larsson, M,

Kukk, E,

Tashir, M,

Osipov, T,

Wada, S,

Salén, P,

Meulen, P. van der,

Bostedt, C,

Feifel, R,

TARANTELLI, Francesco,

Thomas, R. D,

Fang, L,

Ueda, K,

Richter, R,

Bozek, J. D,

Schmidt, H. T,

Ehara, M

2012

Overview

We use extremely intense, ultrashort soft X-Ray pulses generated by the LCLS X-Ray Free Electron Laser to investigate the production of molecular double core-hole states by sequential two-photon X-Ray absorption. The effect of critical LCLS parameters such as the number of photons per pulse, the pulse duration, and the focal spot size on the photoelectron and Auger spectra is modeled in detail and the results of these simulations are used as an aid in the interpretation of the experimental spectra obtained. The emphasis is on double core-hole formation in small polyatomic molecules such as CO2.

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Publisher

IOP Publishing

Subject

Auger spectrum; Core-hole state; Experimental spectra; Focal spot size; Polyatomic molecules; Pulse durations; Soft x-ray pulse; Two photon; X-ray free electron lasers; Carbon dioxide; Free electron lasers; Molecules; Photoelectron spectroscopy

/ Augers

/ Carbon dioxide

/ Formations

/ Free electron lasers

/ Photoelectrons

/ Photons