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Observation of photo-induced plasmon–phonon coupling in PbTe via ultrafast x-ray scattering
Observation of photo-induced plasmon–phonon coupling in PbTe via ultrafast x-ray scattering
by Hauber, A. , Hoffmann, M. C. , Savić, I. , Chollet, M. , Murray, É. D. , Reis, D. A. , Merlin, R. , Zhu, D. , May, A. F. , Clark, J. N. , Henighan, T. , Lindenberg, A. M. , Bray, C. , Zalden, P. , Trigo, M. , Jiang, M. P. , Kozina, M. , Glownia, J. M. , Sato, T. , Sales, B. C. , Delaire, O. , Fahy, S.
2022
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Observation of photo-induced plasmon–phonon coupling in PbTe via ultrafast x-ray scattering
by Hauber, A. , Hoffmann, M. C. , Savić, I. , Chollet, M. , Murray, É. D. , Reis, D. A. , Merlin, R. , Zhu, D. , May, A. F. , Clark, J. N. , Henighan, T. , Lindenberg, A. M. , Bray, C. , Zalden, P. , Trigo, M. , Jiang, M. P. , Kozina, M. , Glownia, J. M. , Sato, T. , Sales, B. C. , Delaire, O. , Fahy, S.
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2022
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Observation of photo-induced plasmon–phonon coupling in PbTe via ultrafast x-ray scattering
Observation of photo-induced plasmon–phonon coupling in PbTe via ultrafast x-ray scattering
by Hauber, A. , Hoffmann, M. C. , Savić, I. , Chollet, M. , Murray, É. D. , Reis, D. A. , Merlin, R. , Zhu, D. , May, A. F. , Clark, J. N. , Henighan, T. , Lindenberg, A. M. , Bray, C. , Zalden, P. , Trigo, M. , Jiang, M. P. , Kozina, M. , Glownia, J. M. , Sato, T. , Sales, B. C. , Delaire, O. , Fahy, S.
2022

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Observation of photo-induced plasmon–phonon coupling in PbTe via ultrafast x-ray scattering
Observation of photo-induced plasmon–phonon coupling in PbTe via ultrafast x-ray scattering
Journal Article

Observation of photo-induced plasmon–phonon coupling in PbTe via ultrafast x-ray scattering

Hauber, A.,
Hoffmann, M. C.,
Savić, I.,
Chollet, M.,
Murray, É. D.,
Reis, D. A.,
Merlin, R.,
Zhu, D.,
May, A. F.,
Clark, J. N.,
Henighan, T.,
Lindenberg, A. M.,
Bray, C.,
Zalden, P.,
Trigo, M.,
Jiang, M. P.,
Kozina, M.,
Glownia, J. M.,
Sato, T.,
Sales, B. C.,
Delaire, O.,
Fahy, S.
2022
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Overview
We report the observation of photo-induced plasmon–phonon coupled modes in the group IV–VI semiconductor PbTe using ultrafast x-ray diffuse scattering at the Linac Coherent Light Source. We measure the near-zone-center excited-state dispersion of the heavily screened longitudinal optical (LO) phonon branch as extracted from differential changes in x-ray diffuse scattering intensity following above bandgap photoexcitation. We suggest that upon photoexcitation, the LO phonon-plasmon coupled (LOPC) modes themselves become coupled to longitudinal acoustic modes that drive electron band shifts via acoustic deformation potentials and possibly to low-energy single-particle excitations within the plasma and that these couplings give rise to displacement-correlations that oscillate in time with a period given effectively by the heavily screened LOPC frequency.
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Publisher
American Institute of Physics,American Crystallographic Association,AIP Publishing LLC and ACA

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