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Stimulated resonant inelastic X-ray scattering in a solid

by Maxwell, Tim , Liu, Tianmin , Dürr, Hermann A. , Higley, Daniel J. , Chase, Tyler , Föhlisch, Alexander , Ding, Yuantao , Mitra, Ankush , Hantschmann, Markus , Stöhr, Joachim , Mehta, Virat , Hellwig, Olav , Kukreja, Roopali , Jal, Emmanuelle , Schlotter, William F. , Chen, Zhao , Beye, Martin , Engel, Robin Y. , Bucher, Maximilian , Carron, Sebastian , Reid, Alex H. , Dakovski, Georgi L. , Bonetti, Stefano

in 639/624/400/1106 / 639/766/119/995 / 639/766/930 / Cobalt / Condensed Matter / Free electron lasers / Inelastic scattering / Luminous intensity / Multilayers / Palladium / Photons / Physics / Physics and Astronomy / Spectrum analysis / Strongly Correlated Electrons / X-ray scattering / X-rays

2022

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2022

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2022

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Journal Article

Stimulated resonant inelastic X-ray scattering in a solid

Maxwell, Tim,

Liu, Tianmin,

Dürr, Hermann A.,

Higley, Daniel J.,

Chase, Tyler,

Föhlisch, Alexander,

Ding, Yuantao,

Mitra, Ankush,

Hantschmann, Markus,

Stöhr, Joachim,

Mehta, Virat,

Hellwig, Olav,

Kukreja, Roopali,

Jal, Emmanuelle,

Schlotter, William F.,

Chen, Zhao,

Beye, Martin,

Engel, Robin Y.,

Bucher, Maximilian,

Carron, Sebastian,

Reid, Alex H.,

Dakovski, Georgi L.,

Bonetti, Stefano

2022

Overview

When materials are exposed to X-ray pulses with sufficiently high intensity, various nonlinear effects can occur. The most fundamental one consists of stimulated electronic decays after resonant absorption of X-rays. Such stimulated decays enhance the number of emitted photons and the emission direction is confined to that of the stimulating incident photons which clone themselves in the process. Here we report the observation of stimulated resonant elastic (REXS) and inelastic (RIXS) X-ray scattering near the cobalt L 3 edge in solid Co/Pd multilayer samples. We observe an enhancement of order 10 6 of the stimulated over the conventional spontaneous RIXS signal into the small acceptance angle of the RIXS spectrometer. We also find that in solids both stimulated REXS and RIXS spectra contain contributions from inelastic electron scattering processes, even for ultrashort 5 fs pulses. Our results reveal the potential and caveats of the development of stimulated RIXS in condensed matter. X-ray free electron lasers provide brilliant light with sufficient intensity to strongly drive and probe nonlinear X-ray-matter interactions. Here, spectroscopy of Co/Pd multilayers reveals a nearly one-million-fold enhancement of stimulated resonant inelastic X-ray scattering versus conventional, spontaneous scattering.

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Publisher

Nature Publishing Group UK,Nature Publishing Group,Nature Research,Nature Portfolio

Subject

/ Cobalt

/ Free electron lasers

/ Inelastic scattering