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Probing the Ultimate Limits of Plasmonic Enhancement

by Ciracì, C. , Maier, S. A. , Fernández-Domínguez, A. I. , Chilkoti, A. , Pendry, J. B. , Mock, J. J. , Hill, R. T. , Urzhumov, Y. , Smith, D. R.

in angle of incidence / Atoms & subatomic particles / Boundaries / Charge density / Collective excitations (including excitons, polarons, plasmons and other charge-density excitations) / Condensed matter: electronic structure, electrical, magnetic, and optical properties / Electric fields / Electronic structure and electrical properties of surfaces, interfaces, thin films and low-dimensional structures / Electronic structure of nanoscale materials : clusters, nanoparticles, nanotubes, and nanocrystals / Electronics / Electrons / Exact sciences and technology / Focusing / Gold - chemistry / Hydrodynamics / Light / Localization / Material films / Materials science / Metal Nanoparticles - chemistry / Metals / Modeling / Nanoparticles / Nanospheres - chemistry / Nanostructure / Nanostructured materials / Nonlinear optics / Optics / Physics / Plasmonics / Plasmons / Resonance scattering / Scattering, Radiation / Surface and interface electron states / Surface Plasmon Resonance / Wavelengths

2012

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Probing the Ultimate Limits of Plasmonic Enhancement

by Ciracì, C. , Maier, S. A. , Fernández-Domínguez, A. I. , Chilkoti, A. , Pendry, J. B. , Mock, J. J. , Hill, R. T. , Urzhumov, Y. , Smith, D. R.

2012

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Probing the Ultimate Limits of Plasmonic Enhancement

by Ciracì, C. , Maier, S. A. , Fernández-Domínguez, A. I. , Chilkoti, A. , Pendry, J. B. , Mock, J. J. , Hill, R. T. , Urzhumov, Y. , Smith, D. R.

2012

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Journal Article

Probing the Ultimate Limits of Plasmonic Enhancement

Ciracì, C.,

Maier, S. A.,

Fernández-Domínguez, A. I.,

Chilkoti, A.,

Pendry, J. B.,

Mock, J. J.,

Hill, R. T.,

Urzhumov, Y.,

Smith, D. R.

2012

Overview

Metals support surface plasmons at optical wavelengths and have the ability to localize light to subwavelength regions. The field enhancements that occur in these regions set the ultimate limitations on a wide range of nonlinear and quantum optical phenomena. We found that the dominant limiting factor is not the resistive loss of the metal, but rather the intrinsic nonlocality of its dielectric response. A semiclassical model of the electronic response of a metal places strict bounds on the ultimate field enhancement. To demonstrate the accuracy of this model, we studied optical scattering from gold nanoparticles spaced a few angstroms from a gold film. The bounds derived from the models and experiments impose limitations on all nanophotonic systems.

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Publisher

American Association for the Advancement of Science,The American Association for the Advancement of Science

Subject

angle of incidence

/ Atoms & subatomic particles

/ Boundaries

/ Charge density

/ Collective excitations (including excitons, polarons, plasmons and other charge-density excitations)

/ Condensed matter: electronic structure, electrical, magnetic, and optical properties

/ Electric fields