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Modulating Propane Dehydrogenation Performance and Stability of Ni.sub.2P with Co Doping
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Modulating Propane Dehydrogenation Performance and Stability of Ni.sub.2P with Co Doping
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Journal Article
Modulating Propane Dehydrogenation Performance and Stability of Ni.sub.2P with Co Doping
2024
Overview
Non-oxidative propane dehydrogenation is an endothermic reaction requiring thermally stable and regenerable catalysts to produce propylene. In this work, we investigate bimetallic Co.sub.XNi.sub.2-XP as an alternative, non-noble metal propane dehydrogenation catalyst. Co.sub.1Ni.sub.1P displayed higher propylene selectivity than Co.sub.2P and higher site-normalized propylene production rates than Ni.sub.2P. Different compositions of Co.sub.XNi.sub.2-XP catalysts were evaluated for propane dehydrogenation with oxidative regeneration in between each cycle. Ni-rich Co.sub.0.5Ni.sub.1.5P showed increased propylene production upon regeneration due to the formation of the Ni.sub.12P.sub.5 phase during reaction. In contrast, Co.sub.1Ni.sub.1P and Co.sub.1.25Ni.sub.0.75P showed the ability to recover > 50% of the initial activity for at least 3 oxidative regenerations, while maintaining high propylene selectivity without any phase change. This study showcases the enhancement in stability and propane dehydrogenation performance of Ni.sub.2P through Co incorporation and Ni:Co ratio control.
Publisher
Springer
Subject
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