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Dehydrocyclization of C.sub.6 Hydrocarbon With and Without Oxygen Containing Substituent Over Pt
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Dehydrocyclization of C.sub.6 Hydrocarbon With and Without Oxygen Containing Substituent Over Pt
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Journal Article
Dehydrocyclization of C.sub.6 Hydrocarbon With and Without Oxygen Containing Substituent Over Pt
2016
Overview
The presence of hydroxyl or keto functional group affects both activity and selectivity for dehydrocyclization of C.sub.6 hydrocarbon over Pt/(Na)-Al.sub.2O.sub.3 catalyst. Under similar reaction conditions, n-hexane produces benzene as the primary product (>40 %), whereas dehydration is a major reaction pathway for 2-hexanol and yields mainly hexenes (>70 %). However, 2-hexanone was found to be involved in a variety of reactions over Pt/(Na)-Al.sub.2O.sub.3 catalyst and produces lower hydrocarbons (C.sub.2-C.sub.5), 5-dodecanone, 2- and 5-nonanones, and 2-acetyl-3-propyl-2-cyclohexen-1-one. The presence of hydroxyl (-OH) or keto group (=C=O) at the C-2 position alters the interaction of C.sub.6 hydrocarbon with the catalyst surface which eventually controls the overall product selectivity.
Publisher
Springer
Subject
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