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Evidence for a glassy state in strongly driven carbon

by Lemke, H. , Neumayer, P. , Moinard, A. , Heimann, P. , Lamb, D. Q. , Fritz, D. , Vinko, S. M. , Plagemann, K. -U. , Rosmej, F. B. , Förster, E. , Sperling, P. , Brown, C. R. D. , White, T. G. , Tschentscher, T. , Toleikis, S. , Wünsch, K. , Cammarata, M. , Fortmann, C. , Galtier, E. , Makita, M. , Döppner, T. , Glenzer, S. H. , Lee, H. J. , Engelhorn, K. , Gregori, G. , Kugland, N. L. , Zhu, D. , Vorberger, J. , Redmer, R. , Gericke, D. O. , Lee, R. W. , Murphy, C. D. , Cho, B. I. , Nagler, B. , Riley, D. , White, S. , Zastrau, U. , Harmand, M.

in INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY

2014

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Evidence for a glassy state in strongly driven carbon

in INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY

2014

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Evidence for a glassy state in strongly driven carbon

in INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY

2014

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Journal Article

Evidence for a glassy state in strongly driven carbon

Lemke, H.,

Neumayer, P.,

Moinard, A.,

Heimann, P.,

Lamb, D. Q.,

Fritz, D.,

Vinko, S. M.,

Plagemann, K. -U.,

Rosmej, F. B.,

Förster, E.,

Sperling, P.,

Brown, C. R. D.,

White, T. G.,

Tschentscher, T.,

Toleikis, S.,

Wünsch, K.,

Cammarata, M.,

Fortmann, C.,

Galtier, E.,

Makita, M.,

Döppner, T.,

Glenzer, S. H.,

Lee, H. J.,

Engelhorn, K.,

Gregori, G.,

Kugland, N. L.,

Zhu, D.,

Vorberger, J.,

Redmer, R.,

Gericke, D. O.,

Lee, R. W.,

Murphy, C. D.,

Cho, B. I.,

Nagler, B.,

Riley, D.,

White, S.,

Zastrau, U.,

Harmand, M.

2014

Overview

Here, we report results of an experiment creating a transient, highly correlated carbon state using a combination of optical and x-ray lasers. Scattered x-rays reveal a highly ordered state with an electrostatic energy significantly exceeding the thermal energy of the ions. Strong Coulomb forces are predicted to induce nucleation into a crystalline ion structure within a few picoseconds. However, we observe no evidence of such phase transition after several tens of picoseconds but strong indications for an over-correlated fluid state. The experiment suggests a much slower nucleation and points to an intermediate glassy state where the ions are frozen close to their original positions in the fluid.

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Nature Publishing Group

Subject

INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY