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$Coulomb explosion imaging of concurrent CH\$_2\$BrI photodissociation dynamics$

Coulomb explosion imaging of concurrent CH\$_2\$BrI photodissociation dynamics

by Journel, Loïc , Ziaee, Farzaneh , Rudenko, Artem , Maclot, Sylvain , Manschwetus, Bastian , Gentleman, Alexander S , Johnsson, Per , Ruchon, Thierry , Rouzée, Arnaud , Bomme, Cédric , Stapelfeldt, Henrik , Mereshchenko, Andrey S , Erk, Benjamin , Treusch, Rolf , Burt, Michael , Holland, David M P , Rolles, Daniel , Boll, Rebecca , Wiese, Joss , Lee, Jason W L , Guillemin, Renaud , Ismail, Iyas , Lahl, Jan , Geneaux, Romain , Maria Novella Piancastelli , Géléoc, Marie , Brausse, Felix , Marchenko, Tatiana , Travnikova, Oksana , Cunha de Miranda, Barbara , Schirmel, Nora , Bari, Sadia , Vallance, Claire , Simon, Marc , Savelyev, Evgeny , Palaudoux, Jérôme , Küpper, Jochen , Brouard, Mark , Trippel, Sebastian , Müller, Erland , Goldsztejn, Gildas , Techert, Simone , Mackenzie, Stuart R , Underwood, Jonathan , Rompotis, Dimitrios , Olshin, Pavel K , Amini, Kasra , Düsterer, Stefan , Köckert, Hansjochen , Penent, Francis

in Charged particles / Explosions / Femtosecond pulses / Imaging / Organic chemistry / Photodissociation

2017

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Coulomb explosion imaging of concurrent CH\$_2\$BrI photodissociation dynamics

in Charged particles / Explosions / Femtosecond pulses / Imaging / Organic chemistry / Photodissociation

2017

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$Coulomb explosion imaging of concurrent CH\$_2\$BrI photodissociation dynamics$

Coulomb explosion imaging of concurrent CH\$_2\$BrI photodissociation dynamics

in Charged particles / Explosions / Femtosecond pulses / Imaging / Organic chemistry / Photodissociation

2017

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$Coulomb explosion imaging of concurrent CH\$_2\$BrI photodissociation dynamics$

Paper

Coulomb explosion imaging of concurrent CH\$_2\$BrI photodissociation dynamics

Journel, Loïc,

Ziaee, Farzaneh,

Rudenko, Artem,

Maclot, Sylvain,

Manschwetus, Bastian,

Gentleman, Alexander S,

Johnsson, Per,

Ruchon, Thierry,

Rouzée, Arnaud,

Bomme, Cédric,

Stapelfeldt, Henrik,

Mereshchenko, Andrey S,

Erk, Benjamin,

Treusch, Rolf,

Burt, Michael,

Holland, David M P,

Rolles, Daniel,

Boll, Rebecca,

Wiese, Joss,

Lee, Jason W L,

Guillemin, Renaud,

Ismail, Iyas,

Lahl, Jan,

Geneaux, Romain,

Maria Novella Piancastelli,

Géléoc, Marie,

Brausse, Felix,

Marchenko, Tatiana,

Travnikova, Oksana,

Cunha de Miranda, Barbara,

Schirmel, Nora,

Bari, Sadia,

Vallance, Claire,

Simon, Marc,

Savelyev, Evgeny,

Palaudoux, Jérôme,

Küpper, Jochen,

Brouard, Mark,

Trippel, Sebastian,

Müller, Erland,

Goldsztejn, Gildas,

Techert, Simone,

Mackenzie, Stuart R,

Underwood, Jonathan,

Rompotis, Dimitrios,

Olshin, Pavel K,

Amini, Kasra,

Düsterer, Stefan,

Köckert, Hansjochen,

Penent, Francis

2017

Overview

The dynamics following laser-induced molecular photodissociation of gas-phase CH\$_2\$BrI at 271.6 nm were investigated by time-resolved Coulomb explosion imaging using intense near-IR femtosecond laser pulses. The observed delay-dependent photofragment momenta reveal that CH\$_2\$BrI undergoes C-I cleavage, depositing 65.6% of the available energy into internal product states, and that absorption of a second UV photon breaks the C-Br bond of CH\$_2\$Br. Simulations confirm that this mechanism is consistent with previous data recorded at 248 nm, demonstrating the sensitivity of Coulomb explosion imaging as a real-time probe of chemical dynamics.

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Publisher

Cornell University Library, arXiv.org

Subject

/ Imaging