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Multi-domain structure: A biomimetic strategy for advanced polymeric materials
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Dissertation
Multi-domain structure: A biomimetic strategy for advanced polymeric materials
2006
Overview
A long lasting challenge in polymer science is to design polymers that combine desired mechanical properties such as tensile strength, fracture toughness, and elasticity into one structure. A novel biomimetic modular polymer design is reported here to address this challenge. Following the molecular mechanism used in nature, modular polymers containing multiple loops were constructed by using precise and strong hydrogen bonding units. Single-molecule force-extension experiments revealed the sequential unfolding of loops as a chain is stretched. The excellent correlation between the single-molecule and the bulk properties successfully demonstrates our biomimetic concept of using modular domain structure to achieve advanced polymer properties.
Publisher
ProQuest Dissertations & Theses
Subject
ISBN
0542997762, 9780542997761
