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Spin and Orbital Rashba effects at the Ni/HfO\\(_2\\) interface
Spin and Orbital Rashba effects at the Ni/HfO\\(_2\\) interface
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Spin and Orbital Rashba effects at the Ni/HfO\\(_2\\) interface
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Spin and Orbital Rashba effects at the Ni/HfO\\(_2\\) interface
Spin and Orbital Rashba effects at the Ni/HfO\\(_2\\) interface
Paper

Spin and Orbital Rashba effects at the Ni/HfO\\(_2\\) interface

2024
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Overview
We predict the giant ferroelectric control of interfacial properties of Ni/HfO2, namely, (i) the magnetocrystalline anisotropy and (ii) the inverse spin and orbital Rashba effects. The reversible control of magnetic properties using electric gating is a promising route to low-energy consumption magnetic devices, including memories and logic gates. Synthetic multiferroics, composed of a ferroelectric in proximity to a magnet, stand out as a promising platform for such devices. Using a combination of \\(ab\\) \\(initio\\) simulations and transport calculations, we demonstrate that reversing the electric polarization modulates the interface magnetocrystalline anisotropy from in-plane to out-of-plane. This modulation compares favorably with recent reports obtained upon electromigration induced by ionic gating. In addition, we find that the current-driven spin and orbital densities at the interface can be modulated by about 50% and 30%, respectively. This giant modulation of the spin-charge and orbit-charge conversion efficiencies opens appealing avenues for voltage-controlled spin- and orbitronics devices.