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The temperature measurement of material inside of an object is one of the key technologies for control of dynamical processes. For this purpose, various techniques such as laser-based thermography and phase-contrast imaging thermography have been studied. However, it is, in principle, impossible to measure the temperature of an element inside of an object using these techniques. One of the possible solutions is measurements of Doppler brooding effect in neutron resonance absorption (NRA). Here we present a method to measure the temperature of an element or an isotope inside of an object using NRA with a single neutron pulse of approximately 100 ns width provided from a high-power laser. We demonstrate temperature measurements of a tantalum (Ta) metallic foil heated from the room temperature up to 617 K. Although the neutron energy resolution is fluctuated from shot to shot, we obtain the temperature dependence of resonance Doppler broadening using a reference of a silver (Ag) foil kept to the room temperature. A free gas model well reproduces the results. This method enables element(isotope)-sensitive thermometry to detect the instantaneous temperature rise in dynamical processes. Non-contact thermometry is one of the key technologies for modern science and industry. Here, authors demonstrated measurement of temperature of an element using neutron resonance spectroscopy with Doppler broadening with single intense short neutron pulse provided from high peak power.

Laser-driven neutron sources (LDNSs) can generate strong short-pulse neutron beams, which are valuable for scientific studies and engineering applications. Neutron resonance transmission analysis (NRTA) is a nondestructive technique used for determining the areal density of each nuclide in a material sample using pulsed thermal and epithermal neutrons. Herein, we report the first successful NRTA performed using an LDNS driven by the Laser for Fast Ignition Experiment at the Institute of Laser Engineering, Osaka University. The key challenge was achieving a well-resolved resonance transmission spectrum for material analysis using an LDNS with a limited number of laser shots in the presence of strong background noise. We addressed this by employing a time-gated 6 Li -glass scintillation neutron detector to measure the transmission spectra, reducing the impact of electromagnetic noise and neutron and gamma-ray flashes. Output waveforms were recorded for each laser shot and analyzed offline using a counting method. This approach yielded a spectrum with distinct resonances, which were attributed to 115 In and 109 Ag , as confirmed through neutron transmission simulation. The spectrum was analyzed using the least-square nuclear-resonance fitting program, REFIT, demonstrating the possibility of using an LDNS for nondestructive areal-density material characterization.

The advance of laser-driven neutron sources (LDNSs) has enabled neutron resonance spectroscopy to be performed with a single shot of a laser. In this study, we describe a detection system of epithermal (∼eV) neutrons especially designed for neutron resonance spectroscopy. A time-gated photomultiplier tube (PMT) with a high cut-off ratio was introduced for epithermal neutron detection in a high-power laser experiment at the Institute of Laser Engineering, Osaka University. We successfully reduced the PMT response to the intense hard X-ray generated as a result of the interaction between laser light and the target material. A time-gated circuit was designed to turn off the response of the PMT during the laser pulse and resume recording the signal when neutrons arrive. The time-gated PMT was coupled with a 6Li glass scintillator, serving as a time-of-flight (TOF) detector to measure the neutron resonance absorption values of 182W and 109Ag in a laser-driven epithermal neutron generation experiment. The neutron resonance peaks at 4.15 eV of 182W and 5.19 eV of 109Ag were detected after a single pulse of laser at a distance of 1.07 m.

We predict the production yield of a medical radioisotope ^{67}$ Cu using ^{67}$ Zn(n, p) ^{67}$ Cu and ^{68}$ Zn(n, pn) ^{67}$ Cu reactions with fast neutrons provided from laser-driven neutron sources. The neutrons were generated by the p+ ^9\\mathrm{Be}$ and d+ ^9$ Be reactions with high-energy ions accelerated by laser–plasma interaction. We evaluated the yield to be (3.3 $\\pm$ 0.5) $\\times$ 10 ^5$ atoms for ^{67}$ Cu, corresponding to a radioactivity of 1.0 $\\pm$ 0.2 Bq, for a Zn foil sample with a single laser shot. Using a simulation with this result, we estimated ^{67}$ Cu production with a high-frequency laser. The result suggests that it is possible to generate ^{67}$ Cu with a radioactivity of 270 MBq using a future laser system with a frequency of 10 Hz and 10,000-s radiation in a hospital.

An amendment to this paper has been published and can be accessed via a link at the top of the paper.

Recent progress of laser science provides laser-driven neutron source (LDNS), which has remarkable features such as the short pulse width. One of the key techniques to be developed for more efficient use of the LDNS is neutron collimation tubes to increase the number of neutrons arriving at a detector in the time-of-flight method. However, when a tube with a thick wall is used as a collimator the neutron collection efficiency at the detector increases but the time resolution becomes wider because of multiple scattering inside of the tube. In the present study, we have developed a collimation tube made of Ni-0, which is optimized for the increased neutron collection efficiency and a reasonable time resolution. This collimator has been demonstrated experimentally using neutron resonance spectroscopy with neutrons provided from LFEX laser.

Generation of quasi-monoenergetic ions by intense laser is one of long-standing goals in laser-plasma physics. However, existing laser-driven ion acceleration schemes often produce broad energy spectra and limited control over ion species. Here we propose the acceleration mechanism, boosted Coulomb explosion, initiated by a standing wave, which is formed in a pre-expanded plasma by the interference between a continuously incoming main laser pulse and the pulse reflected by a solid target, where the pre-expanded plasma is formed from a thin layer on the solid target by a relatively strong pre-pulse. This mechanism produces a persistent Coulomb field on the target front side with field strengths on the order of TV/m for picoseconds. We experimentally demonstrate generation of quasi-monoenergetic deuterons up to 50 MeV using an in-situ D\\(_2\\)O-deposited target. Our results show that the peak energy can be tuned by the laser pulse duration.

Generation of quasi-monoenergetic ion pulse by laser-driven acceleration is one of the hot topics in laser plasma physics. In this study, we present a new method for the \\textit{In-situ} deposition of an ultra-thin D\\(_2\\)O layer on the surface of an aluminum foil target utilizing a spherical D\\(_2\\)O capsule. Employing a 10\\(^{19}\\) W/cm\\(^2\\) laser, we achieve the acceleration of 10.8 MeV deuterons with an energy spread of \\(\\Delta\\)E/E = 4.6% in the most favorable shot. The energy spread depends on the exposure time of the D\\(_2\\)O capsule in the vacuum chamber. This method has the potential to extend its applicability to other ion species.