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Synthesis and Analysis of Temperature-Driven Charge Transport and Dielectric Relaxation in Cs2AgFeCl6 Double Perovskite Single Crystal

by Kumar, Upendra , Patel, Shiv P. , Bhasker, Hari. P. , Dhawan, Punit K. , Kumar, Manvendra , Chaudhary, Dhirendra K. , Yadav, Jitendra , Sharma, Anil K. , Rajput, Parasmani

in Behavior / Charge transport / Chemistry and Materials Science / Chloride / Dielectric properties / Dielectric relaxation / Electronics and Microelectronics / Glass substrates / Instrumentation / Lead / Lead free / Materials Science / Optical and Electronic Materials / Optoelectronic devices / Perovskites / Regular Paper / Single crystals / Spectrum analysis / Temperature / Temperature dependence / Toxicity

2025

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Synthesis and Analysis of Temperature-Driven Charge Transport and Dielectric Relaxation in Cs2AgFeCl6 Double Perovskite Single Crystal

by Kumar, Upendra , Patel, Shiv P. , Bhasker, Hari. P. , Dhawan, Punit K. , Kumar, Manvendra , Chaudhary, Dhirendra K. , Yadav, Jitendra , Sharma, Anil K. , Rajput, Parasmani

2025

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Synthesis and Analysis of Temperature-Driven Charge Transport and Dielectric Relaxation in Cs2AgFeCl6 Double Perovskite Single Crystal

by Kumar, Upendra , Patel, Shiv P. , Bhasker, Hari. P. , Dhawan, Punit K. , Kumar, Manvendra , Chaudhary, Dhirendra K. , Yadav, Jitendra , Sharma, Anil K. , Rajput, Parasmani

2025

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Journal Article

Synthesis and Analysis of Temperature-Driven Charge Transport and Dielectric Relaxation in Cs2AgFeCl6 Double Perovskite Single Crystal

Kumar, Upendra,

Patel, Shiv P.,

Bhasker, Hari. P.,

Dhawan, Punit K.,

Kumar, Manvendra,

Chaudhary, Dhirendra K.,

Yadav, Jitendra,

Sharma, Anil K.,

Rajput, Parasmani

2025

Overview

We successfully grew single crystals of Cs 2 AgFeCl 6 double perovskite measuring ~ 12 mm×01 mm using the acid precipitation method. The dielectric relaxation and charge conduction mechanism has been investigated using temperature-dependent impedance spectroscopy correlated with modulus spectroscopy. We observed the temperature-dependent transition relaxation mechanism from non-Debye-type to Debye-type and the negative temperature coefficient of resistance (NTCR)-type characteristics in Cs 2 AgFeCl 6 single crystals. Moreover, a significant change in dielectric properties, loss factor, electric modulus, and conductivity with temperature has been observed. This investigation provides essential insights into dielectric relaxation behaviour. It elucidates the carrier conduction mechanisms in Cs 2 AgFeCl 6 lead-free double perovskite single crystals that will help design a new optoelectronic device class.

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Publisher

The Korean Institute of Electrical and Electronic Material Engineers (KIEEME),Springer Nature B.V

Subject

Behavior

/ Charge transport

/ Chemistry and Materials Science

/ Chloride

/ Dielectric properties

/ Dielectric relaxation

/ Electronics and Microelectronics