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Catalyst deactivation and regeneration in low temperature ethanol steam reforming with Rh/CeO2–ZrO2 catalysts
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Catalyst deactivation and regeneration in low temperature ethanol steam reforming with Rh/CeO2–ZrO2 catalysts
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Journal Article
Catalyst deactivation and regeneration in low temperature ethanol steam reforming with Rh/CeO2–ZrO2 catalysts
2006
Overview
Rh/CeO2–ZrO2 catalysts with various CeO2/ZrO2 ratios have been applied to H2 production from ethanol steam reforming at low temperatures. The catalysts all deactivated with time on stream (TOS) at 350 °C. The addition of 0.5% K has a beneficial effect on catalyst stability, while 5% K has a negative effect on catalytic activity. The catalyst could be regenerated considerably even at ambient temperature and could recover its initial activity after regeneration above 200 °C with 1% O2. The results are most consistent with catalyst deactivation due to carbonaceous deposition on the catalyst.
Publisher
Springer,Springer Nature B.V
Subject
