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Intrinsically energy-dependent spin dynamics in ultrafast demagnetization
by
Uehlein, Markus
, Held, Tobias
, Rethfeld, Baerbel
, Seibel, Christopher
, Weber, Sebastian T.
in
639/624/400/584
/ 639/766/119/1001
/ 639/766/119/2793
/ 639/766/400/1101
/ Band structure of solids
/ Electrons
/ Energy
/ Equilibrium
/ Lasers
/ Magnetization
/ Optics
/ Physics
/ Physics and Astronomy
/ Spin dynamics
/ Temperature
2025
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Intrinsically energy-dependent spin dynamics in ultrafast demagnetization
by
Uehlein, Markus
, Held, Tobias
, Rethfeld, Baerbel
, Seibel, Christopher
, Weber, Sebastian T.
in
639/624/400/584
/ 639/766/119/1001
/ 639/766/119/2793
/ 639/766/400/1101
/ Band structure of solids
/ Electrons
/ Energy
/ Equilibrium
/ Lasers
/ Magnetization
/ Optics
/ Physics
/ Physics and Astronomy
/ Spin dynamics
/ Temperature
2025
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Do you wish to request the book?
Intrinsically energy-dependent spin dynamics in ultrafast demagnetization
by
Uehlein, Markus
, Held, Tobias
, Rethfeld, Baerbel
, Seibel, Christopher
, Weber, Sebastian T.
in
639/624/400/584
/ 639/766/119/1001
/ 639/766/119/2793
/ 639/766/400/1101
/ Band structure of solids
/ Electrons
/ Energy
/ Equilibrium
/ Lasers
/ Magnetization
/ Optics
/ Physics
/ Physics and Astronomy
/ Spin dynamics
/ Temperature
2025
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Intrinsically energy-dependent spin dynamics in ultrafast demagnetization
Journal Article
Intrinsically energy-dependent spin dynamics in ultrafast demagnetization
2025
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Overview
Ultrafast magnetization dynamics has the potential to spark a new era of information technology by harnessing the interaction between spin and light. Recent studies indicate a complex interplay between the microscopic spin and band structure dynamics and the magneto-optical signals, which are typically exploited in experiments. Using a kinetic model based on microscopic Boltzmann collision integrals, we demonstrate that the spin dynamics are intrinsically energy-dependent due to the non-equilibrium dynamics of carrier distributions and the band structure. We find that the energy-resolved spin dynamics of unoccupied states (holes) differs strongly from those of the electrons. This has major implications for the magneto-optical response, which we reveal to be determined by hole dynamics on early timescales and by electron dynamics on longer timescales.
Energy-resolved optical experiments of ultrafast magnetization dynamics indicate a complex interplay between the spin and band structure dynamics and the magneto-optical signal. In this paper, the authors demonstrate that the spin dynamics are intrinsically energy-dependent and that the magneto-optical response is determined by nonequilibrium hole dynamics on early timescales.
Publisher
Nature Publishing Group UK,Nature Publishing Group,Nature Portfolio
Subject
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