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A comprehensive multidisciplinary investigation on CO2 capture from diesel engine
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Journal Article
A comprehensive multidisciplinary investigation on CO2 capture from diesel engine
2022
Overview
Climate change and global warming are the visible consequences of the increased amount of carbon dioxide (CO
2
) in the atmosphere. Among the various sources of anthropogenic CO
2
emission, the diesel engine has a significant contribution. The development of a reliable system to efficiently minimize CO
2
emissions from diesel engines to the safest level is lacking in the open literature. Therefore, a comprehensive multidisciplinary approach has been applied in this paper to investigate the efficacy of the post-combustion carbon capture (PCC) process for the diesel engine. The experiments have been performed on the exhaust of a direct injection diesel engine at five different brake powers with blends of aqueous ammonia (AQ_NH
3
), monoethanolamine (MEA),
N
,
N
-dimethylethanolamine (DMEA), and 1-ethyl-3-methylimidazolium tetrafluoroborate (C
2
mim BF
4
) ionic liquid (IL) as an absorbent for CO
2
capture. The reaction mechanism of these absorbent with CO
2
are also studied by the geometrical, energetical, MESP, frontier molecular orbitals, and NBO analysis using the first-principles density functional theory (DFT) calculations. The maximum CO
2
absorption efficiency of almost 97% was achieved for the blend consisting of 67% of AQ_NH
3
and 33% of MEA. Moreover, AQ_MEA and blend of AQ_NH
3
, DMEA, and C
2
mim BF
4
ionic liquid showed 96% and 94% CO
2
absorption efficiency, respectively.
Publisher
Springer Berlin Heidelberg,Springer Nature B.V
