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Modulation of the lower critical solution temperature of 2-Alkyl-2-oxazoline copolymers
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Modulation of the lower critical solution temperature of 2-Alkyl-2-oxazoline copolymers
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Journal Article
Modulation of the lower critical solution temperature of 2-Alkyl-2-oxazoline copolymers
2008
Overview
Living cationic copolymerization of 2-isopropyl-2-oxazoline with 2-
n
-propyl-, 2-
n
-butyl-, and 2-
n
-nonyl-2-oxazoline results in gradient copolymers of defined composition, narrow molar mass distributions (PDI = 1.09–1.3), and defined overall degree of polymerization, set to
n
= 25 for all polymers. The introduction of monomer units of stronger amphiphilic character results in a systematic decrease of the lower critical solution temperature (LCST). The LCST modulation can be controlled by the choice of the comonomer as well as the comonomer ratio and was tuned in the temperature range from 46 to 9 °C.
Publisher
Springer-Verlag,Springer,Springer Nature B.V
Subject
/ Cationic
/ Characterization and Evaluation of Materials
/ Chemistry and Materials Science
/ Complex Fluids and Microfluidics
/ Exact sciences and technology
/ Monomers
/ Nanotechnology and Microengineering
/ Physicochemistry of polymers
/ Preparation, kinetics, thermodynamics, mechanism and catalysts
