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Multifunctional roles of carbon‐based hosts for Li‐metal anodes: A review
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Multifunctional roles of carbon‐based hosts for Li‐metal anodes: A review
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Multifunctional roles of carbon‐based hosts for Li‐metal anodes: A review
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Journal Article
Multifunctional roles of carbon‐based hosts for Li‐metal anodes: A review
2021
Overview
With its high theoretical capacity, lithium (Li) metal is recognized as the most potential anode for realizing a high‐performance energy storage system. A series of questions (severe safety hazard, low Coulombic efficiency, short lifetime, etc.) induced by uncontrollable dendrites growth, unstable solid electrolyte interface layer, and large volume change, make practical application of Li‐metal anodes still a threshold. Due to their highly appealing properties, carbon‐based materials as hosts to composite with Li metal have been passionately investigated for improving the performance of Li‐metal batteries. This review displays an overview of the critical role of carbon‐based hosts for improving the comprehensive performance of Li‐metal anodes. Based on correlated mainstream models, the main failure mechanism of Li‐metal anodes is introduced. The advantages and strategies of carbon‐based hosts to address the corresponding challenges are generalized. The unique function, existing limitation, and recent research progress of key carbon‐based host materials for Li‐metal anodes are reviewed. Finally, a conclusion and an outlook for future research of carbon‐based hosts are presented. This review is dedicated to summarizing the advances of carbon‐based materials hosts in recent years and providing a reference for the further development of carbon‐based hosts for advanced Li‐metal anodes. Graphical Carbon‐based hosts are of great significance for the future development of high‐performance Li‐metal anodes. This review summarizes the recent developments of carbon‐based hosts for Li‐metal accommodation. The carbon‐based hosts with high surface area and conductivity can suppress dendrites growth, relieve volume expansion, and stabilize interface, and further doping and compositing to the hosts can effectively regulate Li plating/stripping behaviors.
