Asset Details
Do you wish to reserve the book?
Carrier multiplication detected through transient photocurrent in device-grade films of lead selenide quantum dots
Hey, we have placed the reservation for you!
By the way, why not check out events that you can attend while you pick your title.
Oops! Something went wrong.
Looks like we were not able to place the reservation. Kindly try again later.
Are you sure you want to remove the book from the shelf?
Carrier multiplication detected through transient photocurrent in device-grade films of lead selenide quantum dots
Do you wish to request the book?
Carrier multiplication detected through transient photocurrent in device-grade films of lead selenide quantum dots
Please be aware that the book you have requested cannot be checked out. If you would like to checkout this book, you can reserve another copy
We have requested the book for you!
Your request is successful and it will be processed during the Library working hours. Please check the status of your request in My Requests.
Oops! Something went wrong.
Looks like we were not able to place your request. Kindly try again later.
Journal Article
Carrier multiplication detected through transient photocurrent in device-grade films of lead selenide quantum dots
2015
Overview
In carrier multiplication, the absorption of a single photon results in two or more electron–hole pairs. Quantum dots are promising materials for implementing carrier multiplication principles in real-life technologies. So far, however, most of research in this area has focused on optical studies of solution samples with yet to be proven relevance to practical devices. Here we report ultrafast electro-optical studies of device-grade films of electronically coupled quantum dots that allow us to observe multiplication directly in the photocurrent. Our studies help rationalize previous results from both optical spectroscopy and steady-state photocurrent measurements and also provide new insights into effects of electric field and ligand treatments on multiexciton yields. Importantly, we demonstrate that using appropriate chemical treatments of the films, extra charges produced by carrier multiplication can be extracted from the quantum dots before they are lost to Auger recombination and hence can contribute to photocurrent of practical devices.
In semiconductors, the absorption of a high energy photon can result in the formation of several charge pairs. Here the authors perform ultrafast photocurrent measurements on thin films to explore how quantum dot couplings and the electric field influence multiexciton photovoltaic devices.
Publisher
Nature Publishing Group UK,Nature Publishing Group,Nature Pub. Group
