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Robust interface and reduced operation pressure enabled by co-rolling dry-process for stable all-solid-state batteries
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Robust interface and reduced operation pressure enabled by co-rolling dry-process for stable all-solid-state batteries
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Journal Article
Robust interface and reduced operation pressure enabled by co-rolling dry-process for stable all-solid-state batteries
2025
Overview
The dry-process is a sustainable and promising fabrication method for all-solid-state batteries by eliminating solvents. However, a pragmatic fabrication design for thin and robust solid-state electrolyte (SSE) layers has not been established. Herein, we report a dry-process approach that enhances mechanical stability of SSE layers from film fabrication to cell operation. By co-rolling thick SSE and positive electrode feeds, a uniform, thin SSE layer (50 µm) and a high loading positive electrode layer (5 mAh cm
−2
) with high active material ratio (80 wt%) are simultaneously achieved. This SSE-positive electrode integrated film exhibits enhanced physical properties and cyclability (> 80% retention after 500 cycles) at low stack pressure (2 MPa) compared to the freestanding counterparts, attributed to reinforced and intimate SSE-positive electrode interface constructed during co-rolling process. Additionally, an all-solid-state pouch cell with high stack-level specific energy (310 Wh kg
−1
) and energy density (805 Wh L
−1
) operating at 30 °C and 5 MPa is demonstrated.
All-solid-state batteries face practical challenges such as sustainable fabrication and low-stack pressure operation. Here, authors develop a modified dry-process technique to yield robust solid electrolyte-electrode interface for practical fabrication and operation of all-solid-state batteries.
Publisher
Nature Publishing Group UK,Nature Publishing Group,Nature Portfolio
Subject
