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Critical Review on cathode–electrolyte Interphase Toward High-Voltage Cathodes for Li-Ion Batteries
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Critical Review on cathode–electrolyte Interphase Toward High-Voltage Cathodes for Li-Ion Batteries
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Journal Article
Critical Review on cathode–electrolyte Interphase Toward High-Voltage Cathodes for Li-Ion Batteries
2022
Overview
HighlightsA critical assessment of cathode–electrolyte interphase (CEI) for high-voltage cathode electrodes in Li-ion cells.Fundamental understanding of why interfacial interphase is important to electrochemical performance and further elaboration on how to design robust CEI interphase.Emerging theoretical simulations and advanced in situ characterizations helps to unveil the mystery of CEI are summarized.The thermal stability window of current commercial carbonate-based electrolytes is no longer sufficient to meet the ever-increasing cathode working voltage requirements of high energy density lithium-ion batteries. It is crucial to construct a robust cathode–electrolyte interphase (CEI) for high-voltage cathode electrodes to separate the electrolytes from the active cathode materials and thereby suppress the side reactions. Herein, this review presents a brief historic evolution of the mechanism of CEI formation and compositions, the state-of-art characterizations and modeling associated with CEI, and how to construct robust CEI from a practical electrolyte design perspective. The focus on electrolyte design is categorized into three parts: CEI-forming additives, anti-oxidation solvents, and lithium salts. Moreover, practical considerations for electrolyte design applications are proposed. This review will shed light on the future electrolyte design which enables aggressive high-voltage cathodes.
Publisher
Springer Nature B.V
