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Tunable Emissive CsPbBr3/Cs4PbBr6 Quantum Dots Engineered by Discrete Phase Transformation for Enhanced Photogating in Field‐Effect Phototransistors
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Tunable Emissive CsPbBr3/Cs4PbBr6 Quantum Dots Engineered by Discrete Phase Transformation for Enhanced Photogating in Field‐Effect Phototransistors
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Journal Article
Tunable Emissive CsPbBr3/Cs4PbBr6 Quantum Dots Engineered by Discrete Phase Transformation for Enhanced Photogating in Field‐Effect Phototransistors
2024
Overview
Precise control of quantum structures in hybrid nanocrystals requires advancements in scientific methodologies. Here, on the design of tunable CsPbBr3/Cs4PbBr6 quantum dots are reported by developing a unique discrete phase transformation approach in Cs4PbBr6 nanocrystals. Unlike conventional hybrid systems that emit solely in the green region, this current strategy produces adjustable luminescence in the blue (450 nm), cyan (480 nm), and green (510 nm) regions with high photoluminescence quantum yields up to 45%, 60%, and 85%, respectively. Concentration‐dependent studies reveal that phase transformation mechanisms and the factors that drive CsBr removal occur at lower dilutions while the dissolution–recrystallization process dominates at higher dilutions. When the polymer‐CsPbBr3/Cs4PbBr6 integrated into a field‐effected transistor the resulting phototransistors featured enhanced photosensitivity exceeding 105, being the highest reported for an n‐type phototransistor, while maintaining good transistor performances as compared to devices consisting of polymer‐CsPbBr3 NCs. This study demonstrates a kinetically controlled discrete phase transformation process that converts non‐luminescent Cs4PbBr6 nanocrystals into hybrid Cs4PbBr6/CsPbBr3 quantum structures emitting blue (430 nm), cyan (480 nm), and green (510 nm) light. The resulting hybrid QDs can be integrated with organic semiconducting polymers to achieve high‐performance n‐type field‐effect phototransistors.
Publisher
John Wiley & Sons, Inc,John Wiley and Sons Inc,Wiley
