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P2-type Na.sub.0.67Mn.sub.0.6Ni.sub.0.3Ti.sub.0.1O.sub.2 as cathode material for sodium-ion batteries: solid electrolyte versus liquid electrolyte
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P2-type Na.sub.0.67Mn.sub.0.6Ni.sub.0.3Ti.sub.0.1O.sub.2 as cathode material for sodium-ion batteries: solid electrolyte versus liquid electrolyte
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P2-type Na.sub.0.67Mn.sub.0.6Ni.sub.0.3Ti.sub.0.1O.sub.2 as cathode material for sodium-ion batteries: solid electrolyte versus liquid electrolyte
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Journal Article
P2-type Na.sub.0.67Mn.sub.0.6Ni.sub.0.3Ti.sub.0.1O.sub.2 as cathode material for sodium-ion batteries: solid electrolyte versus liquid electrolyte
2025
Overview
P2-type Na.sub.0.67Mn.sub.0.6Ni.sub.0.3Ti.sub.0.1O.sub.2 is synthesized via a sol-gel method and its electrochemical performance is investigated as a cathode material for sodium-ion batteries (SIBs) employing both a Na.sub.3Zr.sub.2Si.sub.2PO.sub.12 solid electrolyte and an organic liquid electrolyte. In the liquid electrolyte cells, the Na.sub.0.67Mn.sub.0.6Ni.sub.0.3Ti.sub.0.1O.sub.2 cathode exhibits a high discharge capacity of 87.5 mAh g.sup.-1, with a capacity retention of 73.2% after 500 cycles at 0.1 C (10 mA g.sup.-1), while in the solid electrolyte cells, a higher discharge capacity of 94.5 mAh g.sup.-1 at 0.1 C and an improved high-rate capacity of 70.8 mAh g.sup.-1 at 2 C are demonstrated. Moreover, stable charge/discharge cycles are observed in the solid electrolyte cells, with a discharge capacity of 75.3 mAh g.sup.-1 and a retention of 60.7% over 100 cycles at 1 C. This work highlights the substantial effect of the electrolyte conditions on the performance of layered oxide cathode materials, providing potential strategies to overcome current challenges for high-performance SIBs.
Publisher
Springer
Subject
