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A Closer Look at the Evolution of Supercooled Cloud Droplet Temperature and Lifetime in Different Environmental Conditions with Implications for Ice Nucleation in the Evaporating Regions of Clouds
A Closer Look at the Evolution of Supercooled Cloud Droplet Temperature and Lifetime in Different Environmental Conditions with Implications for Ice Nucleation in the Evaporating Regions of Clouds
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A Closer Look at the Evolution of Supercooled Cloud Droplet Temperature and Lifetime in Different Environmental Conditions with Implications for Ice Nucleation in the Evaporating Regions of Clouds
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A Closer Look at the Evolution of Supercooled Cloud Droplet Temperature and Lifetime in Different Environmental Conditions with Implications for Ice Nucleation in the Evaporating Regions of Clouds
A Closer Look at the Evolution of Supercooled Cloud Droplet Temperature and Lifetime in Different Environmental Conditions with Implications for Ice Nucleation in the Evaporating Regions of Clouds

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A Closer Look at the Evolution of Supercooled Cloud Droplet Temperature and Lifetime in Different Environmental Conditions with Implications for Ice Nucleation in the Evaporating Regions of Clouds
A Closer Look at the Evolution of Supercooled Cloud Droplet Temperature and Lifetime in Different Environmental Conditions with Implications for Ice Nucleation in the Evaporating Regions of Clouds
Journal Article

A Closer Look at the Evolution of Supercooled Cloud Droplet Temperature and Lifetime in Different Environmental Conditions with Implications for Ice Nucleation in the Evaporating Regions of Clouds

2023
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Overview
This study investigates the evolution of temperature and lifetime of evaporating, supercooled cloud droplets considering initial droplet radius ( r 0 ) and temperature ( ), and environmental relative humidity (RH), temperature ( T ∞ ), and pressure ( P ). The time ( t ss ) required by droplets to reach a lower steady-state temperature ( T ss ) after sudden introduction into a new subsaturated environment, the magnitude of Δ T = T ∞ − T ss , and droplet survival time ( t st ) at T ss are calculated. The temperature difference (Δ T ) is found to increase with T ∞ , and decrease with RH and P . Δ T was typically 1–5 K lower than T ∞ , with highest values (∼10.3 K) for very low RH, low P , and T ∞ closer to 0°C. Results show that t ss is <0.5 s over the range of initial droplet and environmental conditions considered. Larger droplets ( r 0 = 30–50 μ m) can survive at T ss for about 5 s to over 10 min, depending on the subsaturation of the environment. For higher RH and larger droplets, droplet lifetimes can increase by more than 100 s compared to those with droplet cooling ignored. T ss of the evaporating droplets can be approximated by the environmental thermodynamic wet-bulb temperature. Radiation was found to play a minor role in influencing droplet temperatures, except for larger droplets in environments close to saturation. The implications for ice nucleation in cloud-top generating cells and near cloud edges are discussed. Using T ss instead of T ∞ in widely used parameterization schemes could lead to enhanced number concentrations of activated ice-nucleating particles (INPs), by a typical factor of 2–30, with the greatest increases (≥100) coincident with low RH, low P , and T ∞ closer to 0°C.