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Preparation of High Flux GO/PS-DVB/PAN Membrane by Filtering Layer-by-Layer Assembly Method for Adsorption of Antibiotics from Water

by Hu, Yacong , Xiong, Yanan , Li, Huiying , Gao, Yuechun , Jia, Zhiqian , Zhu, Yanping , Wang, Xin , Zhang, Xu , Guo, Yuexin , Liu, Chunyan , Chen, Yonghao

in Adsorbents / Adsorption / Antibiotics / Aqueous solutions / Chemistry / Chemistry and Materials Science / Divinylbenzene / Ethanol / Filtration / Graphene / High-performance liquid chromatography / Industrial applications / Inorganic Chemistry / Kinetics / Membranes / Organic Chemistry / Polyacrylonitrile / Polymer Sciences / Polystyrene resins / Reagents / Substrates / Surface water / Vacuum filtration / Water purification

2023

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Preparation of High Flux GO/PS-DVB/PAN Membrane by Filtering Layer-by-Layer Assembly Method for Adsorption of Antibiotics from Water

by Hu, Yacong , Xiong, Yanan , Li, Huiying , Gao, Yuechun , Jia, Zhiqian , Zhu, Yanping , Wang, Xin , Zhang, Xu , Guo, Yuexin , Liu, Chunyan , Chen, Yonghao

2023

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Preparation of High Flux GO/PS-DVB/PAN Membrane by Filtering Layer-by-Layer Assembly Method for Adsorption of Antibiotics from Water

by Hu, Yacong , Xiong, Yanan , Li, Huiying , Gao, Yuechun , Jia, Zhiqian , Zhu, Yanping , Wang, Xin , Zhang, Xu , Guo, Yuexin , Liu, Chunyan , Chen, Yonghao

2023

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Journal Article

Preparation of High Flux GO/PS-DVB/PAN Membrane by Filtering Layer-by-Layer Assembly Method for Adsorption of Antibiotics from Water

Hu, Yacong,

Xiong, Yanan,

Li, Huiying,

Gao, Yuechun,

Jia, Zhiqian,

Zhu, Yanping,

Wang, Xin,

Zhang, Xu,

Guo, Yuexin,

Liu, Chunyan,

Chen, Yonghao

2023

Overview

The poor filtration properties of graphene oxide (GO) membrane limit its application in industry. Graphene oxide/polystyrene-divinylbenzene (PS-DVB) membranes were prepared by vacuum filtering layer-by-layer assembly method on a polyacrylonitrile (PAN) substrate membrane. The adsorption kinetics, adsorption isotherm and permeation performance of tetracycline (TC) and ciprofloxacin (CIP) in aqueous solution on the GO/PS-DVB/PAN membranes were investigated. The results revealed that the adsorption of two antibiotics fitted well with pseudo-second-order kinetics model and Langmuir isothermal adsorption model, with the maximum adsorption capacities of 22.79 and 46.69 mg g −1 for TC and CIP, respectively. The adsorption process was dominated by chemical adsorption. The results of membrane permeability showed that GO/PS-DVB/PAN membrane had high water flux, and the retention rate of antibiotics reached 100%. A high performance liquid chromatography method for determination of antibiotics was also established and the methodology was investigated. The GO/PS-DVB/PAN membrane has broad application prospect for removing antibiotics from water.

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Publisher

Springer US,Springer Nature B.V

Subject

/ Chemistry and Materials Science

/ Divinylbenzene