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Boosting the visible-light activity of ZrO2/g-C3N4 by controlling the crystal structure of ZrO2
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Journal Article
Boosting the visible-light activity of ZrO2/g-C3N4 by controlling the crystal structure of ZrO2
2021
Overview
ZrO
2
/g-C
3
N
4
semiconductor photocatalytic materials were prepared by ultrasonic method. The effect of zirconia with different crystal structure on visible light photocatalytic activity of ZrO
2
/g-C
3
N
4
composite was investigated. Loading monoclinic and tetragonal mixed crystals ZrO
2
can improve the photocatalytic degradation efficiency of g-C
3
N
4
. The optimum composite with 15 wt% ZrO
2
/g-C
3
N
4
showed the superior photocatalytic activity for degradation of RhB and PNP under visible-light irradiation, which are 2.5 and 2.8 times higher than pure g-C
3
N
4
under same conditions. The main active species affecting photocatalytic degradation are holes (h
VB
+
) and ·O
2
−
by photocatalytic active species capture experiment, ·OH is also partially involved in the photocatalytic degradation. The 15 wt% ZrO
2
/g-C
3
N
4
has excellent catalytic performance and good stability in photocatalytic repeated experiments, and has a broad application prospect.
Graphic abstract
Publisher
Springer International Publishing,Springer Nature B.V
Subject
