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Research progress in failure mechanisms and electrolyte modification of high‐voltage nickel‐rich layered oxide‐based lithium metal batteries
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Research progress in failure mechanisms and electrolyte modification of high‐voltage nickel‐rich layered oxide‐based lithium metal batteries
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Journal Article
Research progress in failure mechanisms and electrolyte modification of high‐voltage nickel‐rich layered oxide‐based lithium metal batteries
2024
Overview
High‐voltage nickel (Ni)‐rich layered oxide‐based lithium metal batteries (LMBs) exhibit a great potential in advanced batteries due to the ultra‐high energy density. However, it is still necessary to deal with the challenges in poor cyclic and thermal stability before realizing practical application where cycling life is considered. Among many improved strategies, mechanical and chemical stability for the electrode electrolyte interface plays a key role in addressing these challenges. Therefore, extensive effort has been made to address the challenges of electrode‐electrolyte interface. In this progress, the failure mechanism of Ni‐rich cathode, lithium metal anode and electrolytes are reviewed, and the latest breakthrough in stabilizing electrode‐electrolyte interface is also summarized. Finally, the challenges and future research directions of Ni‐rich LMBs are put forward. Lithium metal batteries show the great potential in advanced batteries due to their ultra‐high energy density. This article discusses the failure mechanisms of Ni‐rich cathodes, lithium metal anodes, and electrolytes, and overviews the latest breakthroughs in stabilizing the electrode electrolyte interface from the aspect of electrolytes.
Publisher
John Wiley & Sons, Inc,Wiley
Subject
