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Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers
Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers
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Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers
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Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers
Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers

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Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers
Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers
Journal Article

Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers

2013
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Overview
Recently, few-femtosecond pulses have become available at hard X-ray free-electron lasers. Coupled with the available sub-10 fs optical pulses, investigations into few-femtosecond dynamics are not far off. However, achieving sufficient synchronization between optical lasers and X-ray pulses continues to be challenging. We report a ‘measure-and-sort’ approach, which achieves sub-10 fs root-mean-squared (r.m.s.) error measurement at hard X-ray FELs, far beyond the 100–200 fs r.m.s. jitter limitations. This timing diagnostic, now routinely available at the Linac Coherent Light Source (LCLS), is based on ultrafast free-carrier generation in optically transparent materials. Correlation between two independent measurements enables unambiguous demonstration of ∼6 fs r.m.s. error in reporting the optical/X-ray delay, with single shot error suggesting the possibility of reaching few-femtosecond resolution. By taking advantage of free-carrier generation in optically transparent media researchers have improved synchronization between optical lasers and free-electron laser pulses. This technique has an optical/X-ray delay with a sub-10 fs r.m.s error.