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Transforming Ti3C2Tx MXene’s intrinsic hydrophilicity into superhydrophobicity for efficient photothermal membrane desalination
by
Wong, Pak Wai
, Wang, Yang
, Jiang, Mengnan
, An, Alicia Kyoungjin
, Guo, Jiaxin
, Zhou, Yongsen
, Wang, Zuankai
, Sun, Jiawei
, Zhang, Baoping
in
147/135
/ 639/4077/909/4101/4103
/ 639/925/357/1018
/ Desalination
/ Distillation
/ Distilled water
/ Energy efficiency
/ Feedwater
/ Heat loss
/ Humanities and Social Sciences
/ Hydrophilicity
/ Hydrophobic surfaces
/ Hydrophobicity
/ Irradiation
/ Membrane processes
/ Membranes
/ multidisciplinary
/ Nanospheres
/ Radiation
/ Repellency
/ Salt rejection
/ Science
/ Science (multidisciplinary)
/ Seawater
/ Self-assembly
/ Spraying
/ Temperature gradients
/ Temperature requirements
/ Vapors
/ Water scarcity
/ Wetting
2022
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Transforming Ti3C2Tx MXene’s intrinsic hydrophilicity into superhydrophobicity for efficient photothermal membrane desalination
by
Wong, Pak Wai
, Wang, Yang
, Jiang, Mengnan
, An, Alicia Kyoungjin
, Guo, Jiaxin
, Zhou, Yongsen
, Wang, Zuankai
, Sun, Jiawei
, Zhang, Baoping
in
147/135
/ 639/4077/909/4101/4103
/ 639/925/357/1018
/ Desalination
/ Distillation
/ Distilled water
/ Energy efficiency
/ Feedwater
/ Heat loss
/ Humanities and Social Sciences
/ Hydrophilicity
/ Hydrophobic surfaces
/ Hydrophobicity
/ Irradiation
/ Membrane processes
/ Membranes
/ multidisciplinary
/ Nanospheres
/ Radiation
/ Repellency
/ Salt rejection
/ Science
/ Science (multidisciplinary)
/ Seawater
/ Self-assembly
/ Spraying
/ Temperature gradients
/ Temperature requirements
/ Vapors
/ Water scarcity
/ Wetting
2022
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Transforming Ti3C2Tx MXene’s intrinsic hydrophilicity into superhydrophobicity for efficient photothermal membrane desalination
by
Wong, Pak Wai
, Wang, Yang
, Jiang, Mengnan
, An, Alicia Kyoungjin
, Guo, Jiaxin
, Zhou, Yongsen
, Wang, Zuankai
, Sun, Jiawei
, Zhang, Baoping
in
147/135
/ 639/4077/909/4101/4103
/ 639/925/357/1018
/ Desalination
/ Distillation
/ Distilled water
/ Energy efficiency
/ Feedwater
/ Heat loss
/ Humanities and Social Sciences
/ Hydrophilicity
/ Hydrophobic surfaces
/ Hydrophobicity
/ Irradiation
/ Membrane processes
/ Membranes
/ multidisciplinary
/ Nanospheres
/ Radiation
/ Repellency
/ Salt rejection
/ Science
/ Science (multidisciplinary)
/ Seawater
/ Self-assembly
/ Spraying
/ Temperature gradients
/ Temperature requirements
/ Vapors
/ Water scarcity
/ Wetting
2022
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Transforming Ti3C2Tx MXene’s intrinsic hydrophilicity into superhydrophobicity for efficient photothermal membrane desalination
Journal Article
Transforming Ti3C2Tx MXene’s intrinsic hydrophilicity into superhydrophobicity for efficient photothermal membrane desalination
2022
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Overview
Owing to its 100% theoretical salt rejection capability, membrane distillation (MD) has emerged as a promising seawater desalination approach to address freshwater scarcity. Ideal MD requires high vapor permeate flux established by cross-membrane temperature gradient (∆T) and excellent membrane durability. However, it’s difficult to maintain constant ∆T owing to inherent heat loss at feedwater side resulting from continuous water-to-vapor transition and prevent wetting transition-induced membrane fouling and scaling. Here, we develop a Ti
3
C
2
T
x
MXene-engineered membrane that imparts efficient localized photothermal effect and strong water-repellency, achieving significant boost in freshwater production rate and stability. In addition to photothermal effect that circumvents heat loss, high electrically conductive Ti
3
C
2
T
x
MXene also allows for self-assembly of uniform hierarchical polymeric nanospheres on its surface via electrostatic spraying, transforming intrinsic hydrophilicity into superhydrophobicity. This interfacial engineering renders energy-efficient and hypersaline-stable photothermal membrane distillation with a high water production rate under one sun irradiation.
Membrane distillation is susceptible to thermal inefficiency and membrane wetting issues during seawater desalination. Here, authors design a MXene-engineered membrane that imparts efficient localized photothermal effect and strong water repellency, achieving sustainable freshwater production.
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