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Room Temperature Deposition of Crystalline Nanoporous ZnO Nanostructures for Direct Use as Flexible DSSC Photoanode
by
Han, Byung Suh
, Sohn, Woonbae
, Lee, Jung-Kun
, Kim, Miyoung
, Caliskan, Salim
, Jang, Ho Won
in
Ablation
/ Chemistry and Materials Science
/ Crystal structure
/ Crystallography
/ Deposition
/ Dye-sensitized solar cells
/ Electrochemical impedance spectroscopy
/ Electrochemistry
/ Electrolytic cells
/ Glass
/ Glass substrates
/ Impurities
/ Materials Science
/ Molecular Medicine
/ Nano Express
/ Nanochemistry
/ Nanoscale Science and Technology
/ Nanostructure
/ Nanotechnology
/ Nanotechnology and Microengineering
/ Photoanodes
/ Photovoltaic cells
/ Polyethylene naphthalate
/ Pulsed laser deposition
/ Pulsed lasers
/ Room temperature
/ Solar cells
/ Spectroscopy
/ Substrates
/ Surface area
/ Zinc oxide
/ Zinc oxides
2016
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Room Temperature Deposition of Crystalline Nanoporous ZnO Nanostructures for Direct Use as Flexible DSSC Photoanode
by
Han, Byung Suh
, Sohn, Woonbae
, Lee, Jung-Kun
, Kim, Miyoung
, Caliskan, Salim
, Jang, Ho Won
in
Ablation
/ Chemistry and Materials Science
/ Crystal structure
/ Crystallography
/ Deposition
/ Dye-sensitized solar cells
/ Electrochemical impedance spectroscopy
/ Electrochemistry
/ Electrolytic cells
/ Glass
/ Glass substrates
/ Impurities
/ Materials Science
/ Molecular Medicine
/ Nano Express
/ Nanochemistry
/ Nanoscale Science and Technology
/ Nanostructure
/ Nanotechnology
/ Nanotechnology and Microengineering
/ Photoanodes
/ Photovoltaic cells
/ Polyethylene naphthalate
/ Pulsed laser deposition
/ Pulsed lasers
/ Room temperature
/ Solar cells
/ Spectroscopy
/ Substrates
/ Surface area
/ Zinc oxide
/ Zinc oxides
2016
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Room Temperature Deposition of Crystalline Nanoporous ZnO Nanostructures for Direct Use as Flexible DSSC Photoanode
by
Han, Byung Suh
, Sohn, Woonbae
, Lee, Jung-Kun
, Kim, Miyoung
, Caliskan, Salim
, Jang, Ho Won
in
Ablation
/ Chemistry and Materials Science
/ Crystal structure
/ Crystallography
/ Deposition
/ Dye-sensitized solar cells
/ Electrochemical impedance spectroscopy
/ Electrochemistry
/ Electrolytic cells
/ Glass
/ Glass substrates
/ Impurities
/ Materials Science
/ Molecular Medicine
/ Nano Express
/ Nanochemistry
/ Nanoscale Science and Technology
/ Nanostructure
/ Nanotechnology
/ Nanotechnology and Microengineering
/ Photoanodes
/ Photovoltaic cells
/ Polyethylene naphthalate
/ Pulsed laser deposition
/ Pulsed lasers
/ Room temperature
/ Solar cells
/ Spectroscopy
/ Substrates
/ Surface area
/ Zinc oxide
/ Zinc oxides
2016
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Room Temperature Deposition of Crystalline Nanoporous ZnO Nanostructures for Direct Use as Flexible DSSC Photoanode
Journal Article
Room Temperature Deposition of Crystalline Nanoporous ZnO Nanostructures for Direct Use as Flexible DSSC Photoanode
2016
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Overview
A facile approach to fabricate dye-sensitized solar cells (DSSCs) is demonstrated by depositing (001) oriented zinc oxide (ZnO) nanostructures on both glass and flexible substrates at room temperature using pulsed laser deposition. Unique crystallographic characteristics of ZnO combined with highly non-equilibrium state of pulsed laser-induced ablated species enabled highly crystalline ZnO nanostructures without aid of any chemically induced additives or organic/inorganic impurities at room temperature. Film morphology as well as internal surface area is tailored by varying ambient oxygen pressure and deposition time. It is revealed that the optimization of these two experimental factors was essential for achieving structure providing large surface area as well as efficient charge collection. The DSSCs with optimized ZnO photoanodes showed overall efficiencies of 3.89 and 3.4 % on glass and polyethylene naphthalate substrates, respectively, under AM 1.5G light illumination. The high conversion efficiencies are attributed to elongated electron lifetime and enhanced electrolyte diffusion in the high crystalline ZnO nanostructures, verified by intensity-modulated voltage spectroscopy and electrochemical impedance measurements.
Publisher
Springer US,Springer Nature B.V
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