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Ferrimagnetism in ionic liquid cation intercalated \\documentclass12pt{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\hbox {NiPS}_3$$\\end{document}
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Journal Article
Ferrimagnetism in ionic liquid cation intercalated \\documentclass12pt{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\hbox {NiPS}_3$$\\end{document}
2025
Overview
The electrochemical intercalation is one of most powerful tools for tuning the intrinsic properties of quasi-two-dimensional (2D) materials. In this work, ionic organic cations, and , are successfully intercalated into interlayer via electrochemical intercalation. The both and intercalated samples show ferrimagnetic transition with the transition temperature of 65 K and 85 K, respectively. Raman spectroscopy, X-ray photoelectron spectroscopy and Hall measurements reveal that the electron doping and sulfur vacancies created by the cation intercalation play important role in the ferrimagnetic transition. Our work provides a new pathway to manipulation of magnetism in layered 2D materials.
Publisher
Nature Publishing Group
